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SFG Investigation of Adsorbed CO and NO on NiO(111) Surface
BANDARA Athula, Shinsaku DOBASHI, Jun KUBOTA, Ken ONDA, Akihide WADA, Kazunari DOMEN, Chiaki HIROSE, Satoru S. KANO
Author information
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BANDARA Athula
Research Laboratory of Resources Utilization, Tokyo Institute of Technology
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Shinsaku DOBASHI
Research Laboratory of Resources Utilization, Tokyo Institute of Technology
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Jun KUBOTA
Research Laboratory of Resources Utilization, Tokyo Institute of Technology
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Ken ONDA
Research Laboratory of Resources Utilization, Tokyo Institute of Technology
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Akihide WADA
Research Laboratory of Resources Utilization, Tokyo Institute of Technology
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Kazunari DOMEN
Research Laboratory of Resources Utilization, Tokyo Institute of Technology
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Chiaki HIROSE
Research Laboratory of Resources Utilization, Tokyo Institute of Technology
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Satoru S. KANO
College of Engineering, Hosei University
JOURNAL
FREE ACCESS
1997 Volume 18 Issue 7 Pages 405-410
Details
- Published: July 10, 1997 Received: January 23, 1997 Available on J-STAGE: August 07, 2009 Accepted: - Advance online publication: - Revised: -
-
Correction information
Date of correction: August 07, 2009 Reason for correction: - Correction: ABSTRACT Details: Wrong : Adsorption structures of CO and NO on the NiO(111) film grown on Ni(111) crystal have been investigated by sum frequency generation (SFG) spectroscopy and infrared reflection absorption spectroscopy (IRAS). The CO stretching band of adsorbed CO on NiO(111) was observed at 2144 cm-1 on the SFG spectra for both p- and s-polarized visible light. However, adsorbed NO on NiO(111) was observed at 1805 cm-1 on the SFG spectra only for the p-polarized visible light. The results suggest that the adsorbed CO molecule was tilted from the surface normal but the NO molecule was perpendicular to the surface. These orientations of CO and NO reflect the surface structure of NiO(111) which has (2×2)reconstructed microfacets. Adsorption of CO on Ni(111) instead of NiO(111) was also examined by SFG and IRAS. Absorption bands due to linear and bridged CO were observed at 2076 and 1918 cm-1, respectively, by IRAS. On the other hand, the linear CO molecules on Ni(111) gave an SFG peak at 2076 cm-1 only for the p-polarized visible light indicating the CO molecules are perpendicular to the surface, and bridged CO molecules did not give any SFG signal. The absence of the bridged CO signal is believed to be due to the smaller Raman tensor of bridged CO.
Right : Adsorption structures of CO and NO on the NiO(111) film grown on Ni(111) crystal have been investigated by sum frequency generation (SFG) spectroscopy and infrared reflection absorption spectroscopy (IRAS). The CO stretching band of adsorbed CO on NiO(111) was observed at 2144 cm-1 on the SFG spectra for both p- and s-polarized visible light. However, adsorbed NO on NiO(111) was observed at 1805 cm-1 on the SFG spectra only for the p-polarized visible light. The results suggest that the adsorbed CO molecule was tilted from the surface normal but the NO molecule was perpendicular to the surface. These orientations of CO and NO reflect the surface structure of NiO(111) which has (2×2)reconstructed microfacets. Adsorption of CO on Ni(111) instead of NiO(111) was also examined by SFG and IRAS. Absorption bands due to linear and bridged CO were observed at 2076 and 1918 cm-1, respectively, by IRAS. On the other hand, the linear CO molecules on Ni(111) gave an SFG peak at 2076 cm-1 only for the p-polarized visible light indicating the CO molecules are perpendicular to the surface, and bridged CO molecules did not give any SFG signal. The absence of the bridged CO signal is believed to be due to the smaller Raman tensor of bridged CO.
Date of correction: August 07, 2009 Reason for correction: - Correction: CITATION Details: Wrong : 1) Y. R. Shen: “The Principles of Nonlinear Optics” (John Wiley & Sons, New York, 1984); Y. R. Shen: Surf. Sci. 299/300,551 (1994).
3) M. Morin, P. Jacob, N. J. Levimos, Y. J. Chabal and A. Harris: J. Chem. Phys. 96, 6203 (1992).
4) H. Yamamoto, N. Akamatsu, A. Wada, K. Domen and C. Hirose: J. Electron Spectrosc. Relat. Phenom. 64/65, 507 (1993).
5) R. Braum, B. D. Casson and C. D. Bain: Chem. Phys. Lett. 245, 326 (1995).
6) P. S. Cremer, X. Su, Y. R. Shen and G. A. Somorjai: J. Am. Chem. Soc. 118, 2942 (1996).
7) A. Peremans and A. Tadjeddine: J. Chem. Phys. 103, 7197 (1995).
8) P. Guyot-Sionnest, P. H. Lin and E. M. Hiller: J. Chem. Phys. 102, 4269 (1995).
9) A. L. Harris, L. Rothberg, L. Dahr, N. J. Levinos and L. H. Dubois: J. Chem. Phys. 94, 2438 (1991).
10) V. E. Henrich and P. A. Cox: “The Surface Science of Metal Oxides” (Cambridge U. P., New York, 1994)
11) M. Bäumer, D. Cappus, H. Kuhlenbeck, H.-J. Freund, G. Wilhelmi, A. Brodde and H. Neddermeyer: Suf. Sci. 253, 116 (1991).
12) C. Xu and D. W. Goodman: J. Chem. Soc. Faraday Trans. 91, 3709 (1995).
13) A. Bandara, J. Kubota, A. Wada, K. Domen and C. Hirose: J. Phys. Chem. 100, 14962 (1996).
14) F. Rohr, K. Wirth, J. Libuda, D. Cappus, M. Bäumer and H.-J. Freund: Surf. Sci. 315, L977 (1994).
15) C. A. Ventrice, Jr., Th. Bertrams, H. Hannemann, A. Brodde and H. Neddermeyer: Phys. Rev. B 49, 5773 (1994).
16) H. Kuhlenbeck, G. Odorfer, R. Jaeger, G. hung, M. Munges, Th. Mull, H. -J. Freund, M. Pohlchen, V. Staemmler, S. Witzel, C. Scharfschwerdt, K. Wennemann, T. Liedtke and M. Neumann: Phys. Rev. B 43, 1969 (1991).
17) A. Bandara, J. Kubota, A. Wada, K. Domen and C. Hirose: J. Phys. Chem. B 101, 361 (1997).
18) M. Schonneback, D. Cappus, J. Klinkmann, H.-J. Freund, L. G. M. Petterson and P. S. Bagus: Surf. Sci. 347, 337 (1996).
20) J. Y. Zhang, J. Y. Huang, Y. R. Shen and C. Chen: J. Opt. Soc. B 10,1758 (1993).
21) J. Yoshinobu, X. Guo and J. T. Yates, Jr.: J. Chem. Phys. 92, 7700 (1991).
22) H. E. Sanders, D. Gardner, D. A. King and M. A. Morris: Surf. Sci. 179, 104 (1994).
23) T. Anzai, H. Maeoka, A. Wada, K. Domen, C. Hirose, T. Ando and Y. Sato: J. Mol. Struct. 352/353, 455 (1995).
24) N. Akamatsu, K. Domen and C. Hirose: J. Phys. Chem. 97, 10064 (1993).
25) M. Born and E. Wolf: “Principle of Optics” (Pergamon Press, Oxford, 1975).
26) W. Suetaka: “Surface Infrared and Raman Spectroscopy” (Plenum, New York, 1995).
27) S. Haq, J. G. Love and D. A. King: Surf. Sci. 275, 170 (1992).
28) M. Trenary, K. J. Uram, F. Bazso and J. T. Yates, Jr.: Surf. Sci. 146, 269 (1984).
29) W. Daum, K. A. Friedrich, C. Kuünker, D. Knabben, U. Stimming and H. Ibach: Appl. Phys. A 59, 553 (1994).
30) J. Miragliotta, R. S. Polizotti, P. Rabinowitz, S. D. Cameron and R. B. Hall: Appl. Phys. A 51, 221 (1990).
31) R. M. Lambert and M. E. Bridge: “The Chemical Physics of Solid Surfaces and Heterogeneous Catalysis Vol. 3” (Elsevier, Amsterdam, 1984).
Right : 1) Y. R. Shen: “The Principles of Nonlinear Optics” (John Wiley & Sons, New York, 1984); Y. R. Shen: Surf. Sci. 299/300,551 (1994).
3) M. Morin, P. Jacob, N. J. Levimos, Y. J. Chabal and A. Harris: J. Chem. Phys. 96, 6203 (1992).
4) H. Yamamoto, N. Akamatsu, A. Wada, K. Domen and C. Hirose: J. Electron Spectrosc. Relat. Phenom. 64/65, 507 (1993).
5) R. Braum, B. D. Casson and C. D. Bain: Chem. Phys. Lett. 245, 326 (1995).
6) P. S. Cremer, X. Su, Y. R. Shen and G. A. Somorjai: J. Am. Chem. Soc. 118, 2942 (1996).
7) A. Peremans and A. Tadjeddine: J. Chem. Phys. 103, 7197 (1995).
8) P. Guyot-Sionnest, P. H. Lin and E. M. Hiller: J. Chem. Phys. 102, 4269 (1995).
9) A. L. Harris, L. Rothberg, L. Dahr, N. J. Levinos and L. H. Dubois: J. Chem. Phys. 94, 2438 (1991).
10) V. E. Henrich and P. A. Cox: “The Surface Science of Metal Oxides” (Cambridge U. P., New York, 1994)
11) M. Bäumer, D. Cappus, H. Kuhlenbeck, H.-J. Freund, G. Wilhelmi, A. Brodde and H. Neddermeyer: Suf. Sci. 253, 116 (1991).
12) C. Xu and D. W. Goodman: J. Chem. Soc. Faraday Trans. 91, 3709 (1995).
13) A. Bandara, J. Kubota, A. Wada, K. Domen and C. Hirose: J. Phys. Chem. 100, 14962 (1996).
14) F. Rohr, K. Wirth, J. Libuda, D. Cappus, M. Bäumer and H.-J. Freund: Surf. Sci. 315, L977 (1994).
15) C. A. Ventrice, Jr., Th. Bertrams, H. Hannemann, A. Brodde and H. Neddermeyer: Phys. Rev. B 49, 5773 (1994).
16) H. Kuhlenbeck, G. Odorfer, R. Jaeger, G. hung, M. Munges, Th. Mull, H. -J. Freund, M. Pohlchen, V. Staemmler, S. Witzel, C. Scharfschwerdt, K. Wennemann, T. Liedtke and M. Neumann: Phys. Rev. B 43, 1969 (1991).
17) A. Bandara, J. Kubota, A. Wada, K. Domen and C. Hirose: J. Phys. Chem. B 101, 361 (1997).
18) M. Schonneback, D. Cappus, J. Klinkmann, H.-J. Freund, L. G. M. Petterson and P. S. Bagus: Surf. Sci. 347, 337 (1996).
20) J. Y. Zhang, J. Y. Huang, Y. R. Shen and C. Chen: J. Opt. Soc. B 10,1758 (1993).
21) J. Yoshinobu, X. Guo and J. T. Yates, Jr.: J. Chem. Phys. 92, 7700 (1991).
22) H. E. Sanders, D. Gardner, D. A. King and M. A. Morris: Surf. Sci. 179, 104 (1994).
23) T. Anzai, H. Maeoka, A. Wada, K. Domen, C. Hirose, T. Ando and Y. Sato: J. Mol. Struct. 352/353, 455 (1995).
24) N. Akamatsu, K. Domen and C. Hirose: J. Phys. Chem. 97, 10064 (1993).
25) M. Born and E. Wolf: “Principle of Optics” (Pergamon Press, Oxford, 1975).
26) W. Suetaka: “Surface Infrared and Raman Spectroscopy” (Plenum, New York, 1995).
27) S. Haq, J. G. Love and D. A. King: Surf. Sci. 275, 170 (1992).
28) M. Trenary, K. J. Uram, F. Bazso and J. T. Yates, Jr.: Surf. Sci. 146, 269 (1984).
29) W. Daum, K. A. Friedrich, C. Kuünker, D. Knabben, U. Stimming and H. Ibach: Appl. Phys. A 59, 553 (1994).
30) J. Miragliotta, R. S. Polizotti, P. Rabinowitz, S. D. Cameron and R. B. Hall: Appl. Phys. A 51, 221 (1990).
31) R. M. Lambert and M. E. Bridge: “The Chemical Physics of Solid Surfaces and Heterogeneous Catalysis Vol. 3” (Elsevier, Amsterdam, 1984).
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